碳酸盐团簇同位素在海相盆地热史研究中的进展

邱楠生; 刘鑫; 熊昱杰; 刘雨晨; 徐秋晨; 常青

doi:10.11781/sysydz202305891

碳酸盐团簇同位素在海相盆地热史研究中的进展

doi: 10.11781/sysydz202305891

邱楠生^{1, 2,},
刘鑫^{1, 2},
熊昱杰^{1, 2},
刘雨晨^{1, 2},
徐秋晨^{1, 2},
常青^{1, 2}

1.
中国石油大学(北京) 油气资源与探测国家重点实验室, 北京 102249
2.
中国石油大学(北京) 地球科学学院, 北京 102249

基金项目:

国家自然科学基金项目 41830424

国家自然科学基金项目 U19B6003

详细信息

作者简介:
邱楠生(1968-), 男, 博士, 教授, 从事盆地构造-热演化研究工作。E-mail: qiunsh@cup.edu.cn

中图分类号: TE135
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出版历程
- 收稿日期: 2023-06-06
- 修回日期: 2023-08-12
- 刊出日期: 2023-09-28

Progress in the study of carbonate clumped isotope in the thermal history of marine basins

QIU Nansheng^{1, 2
,},
LIU Xin^{1, 2},
XIONG Yujie^{1, 2},
LIU Yuchen^{1, 2},
XU Qiuchen^{1, 2},
CHANG Qing^{1, 2}

1.
State Key Laboratory of Petroleum Resources and Prospecting, China University of Petroleum (Beijing), Beijing 102249, China
2.
College of Geosciences, China University of Petroleum (Beijing), Beijing 102249, China

摘要

摘要: 沉积盆地热史研究对于油气成藏分析至关重要，在油气勘探以及油气资源评价领域有着举足轻重的影响，而海相盆地碳酸盐岩层系由于缺乏有效古温标导致很难对其热史进行恢复。碳酸盐团簇同位素是能够指示碳酸盐岩形成温度的指标，它将温度信息记录在¹³C—¹⁸O配对的化学键中，并通过其丰度变化将温度信息反映出来，即碳酸盐团簇同位素的丰度(Δ₄₇)与地层温度演化密切相关。从碳酸盐团簇同位素测温以及热史恢复的基本原理、方法出发，结合近年来其在国内外海相盆地热史恢复的研究实例，综述了碳酸盐团簇同位素古温标的应用情况，并探讨了其存在的问题和未来的发展方向。碳酸盐团簇同位素作为一种新兴的古温标，在碳酸盐岩地层热历史恢复中展现出了巨大的潜力。团簇同位素热史研究实例表明，美国箭峡Bird Spring组经历的最高古温度约为175 ℃，四川盆地二叠系茅口组最高埋藏温度在213~225 ℃，塔里木盆地奥陶系受二叠纪岩浆活动影响存在160 ℃以上的异常高温。团簇同位素由于受热演化模式不成熟，重结晶作用以及沉积埋藏温度变化的影响，使得其在热史恢复方面仍存在不足，并建议精确恢复碳酸盐岩地层热史的下一步发展方向是将碳酸盐团簇同位素和U-Pb定年以及其他古温标相联合。
- 团簇同位素 /
- 碳酸盐岩 /
- 海相盆地 /
- 热历史 /
- 塔里木盆地 /
- 四川盆地
Abstract: The study of thermal history of sedimentary basins is very important for oil-gas accumulation analysis and has decisive influence on oil and gas exploration and oil-gas resource evaluation. However, it is difficult to reconstruct the thermal history of carbonate strata in marine basins due to the lack of effective palaeo-thermometer. The carbonate cluster isotope is an index that can indicate the formation temperature of carbonate rock. It records temperature information in chemical bond through conjugated ¹³C-¹⁸O, and temperature information is revealed through changes in the abundance of conjugated ¹³C-¹⁸O, namely, the abundance of carbonate clumped isotope (Δ₄₇) is closely related to the evolution of strata temperature. This paper reviews the application of carbonate clumped isotope palaeo-thermometer and discusses the existing problems and future development direction based on the basic principle and methods of carbonate clumped isotope thermometry and thermal history reconstruction, and combined with the case studies of thermal history reconstruction in marine basins in recent years. As a new palaeo-thermometer, carbonate clumped isotope shows great potential in the thermal history reconstruction of carbonate strata. Previous studies show that the maximum paleotemperature of the Bird Spring Formation in Arrow Canyon, Nevada, USA is about 175 ℃, and the maximum burial temperature of Permian Maokou Formation in the Sichuan Basin is 213-225 ℃. There is an abnormal high temperature of above 160 ℃ in the Ordovician strata of the Tarim Basin due to the Permian magmatic activity. We believe that the carbonate clumped isotope is still insufficient in the reconstruction of thermal history due to the immaturity of thermal evolution models, the recrystallization, and the change of burial temperature. Thus, we suggest that combining the carbonate clumped isotope, U-Pb dating, and other palaeo-thermometers to accurately reconstruct the thermal history of carbonate strata will be the future development direction.
- clumped isotope /
- carbonate strata /
- marine basin /
- thermal history /
- Tarim Basin /
- Sichuan Basin
注释:

利益冲突声明/Conflict of Interests

所有作者声明不存在利益冲突。

All authors disclose no relevant conflict of interests.

作者贡献/Authors’ Contributions

邱楠生和刘鑫负责论文撰写和修改及图件清绘，徐秋晨、常青参与论文写作；刘鑫、熊昱杰、刘雨晨负责塔里木和四川盆地团簇同位素热史恢复的研究；所有作者均阅读并同意最终稿件的提交。

QIU Nansheng and LIU Xin drafted and revised the manuscript and drew the diagrams. XU Qiuchen and CHANG Qing participated in drafting the manuscript. The thermal history of the Tarim and Sichuan basins were modelled by LIU Xin, XIONG Yujie and LIU Yuchen, using clumped-isotope thermal indicators. All the authors have read the last version of paper and consented for submission.

HTML全文

图 1 碳酸盐团簇同位素示意^[12]

Figure 1. Schematic diagram of carbonate clumped isotope

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图 2 一阶近似模型预测的T(Δ₄₇)—埋藏温度图^[31]

Figure 2. Schematic diagram of T(Δ₄₇)-burial T trajectories predicted by first-order approximation model

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图 3 热史路径和最高古温度对碳酸盐中¹³C—¹⁸O键重排和T(Δ₄₇)值的影响示意^[41]

Figure 3. Impact of thermal history path and maximum paleotemperature on ¹³C-¹⁸O bond reordering and T(Δ₄₇) in carbonate

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图 4 美国内华达州箭峡Bird Spring组腕足化石团簇同位素热史恢复结果

图 4a, 4b据文献[31], 4c据文献[24]。

Figure 4. Thermal history reconstructed by clumped isotope of brachiopod fossil from Bird Spring Formation in Arrow Canyon, Nevada, USA

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图 5 美国特拉华盆地不同地温梯度最佳拟合路径模拟^[25]

a图为埋藏史; b图为不同地温梯度下T(Δ₄₇)演化曲线，黑带表示95%可信度。

Figure 5. Best fitting path of different geothermal gradients in Delaware Basin, USA

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图 6 塔中北部斜坡构造带TZ35井碳酸盐团簇同位素温度模拟^[52]

Figure 6. Modeling results of carbonate clumped isotope temperature in well TZ35 on the northern slope of Tazhong Uplift

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图 7 利用交换/扩散模型模拟的塔里木盆地顺托果勒地区团簇同位素温度热模拟结果^[27]

Figure 7. Thermal modeling results of clumped isotope temperature in Shuntuoguole area, Tarim Basin using exchange-diffusion model

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图 8 川东二叠系茅口组钻井样品团簇同位素对地层温度的热模拟结果

Figure 8. Thermal modeling results of clumped isotope of drilling sample from Permian Maokou Formation in eastern Sichuan Basin on strata temperature

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图 9 四川盆地普光气田白云岩团簇同位素温度演化过程^[55]

D83、D89和D99分别代表白云石样品的T(Δ₄₇)及其误差。

Figure 9. Evolution of clumped isotope temperature of dolostone from Puguang Gas Field, Sichuan Basin

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图 10 基于包裹体宿主矿物年龄、团簇同位素温度约束的川中古隆起震旦系灯影组温度演化^[57]

Figure 10. Temperature evolution of Sinian Dengying Formation in paleo-uplift in central Sichuan Basin based on the constraints of the age of the host mineral of the inclusion and the clumped isotope temperature

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